To solve the question regarding the correct statement when adsorption of gas takes place on a metal surface, we will analyze each option step by step.
### Step 1: Analyze Statement (a)
**Statement (a):** `ΔH` becomes less negative with the progress of the reaction.
- When a gas adsorbs onto a metal surface, the randomness (entropy) of the gas molecules decreases because they are confined to the surface.
- Since the entropy decreases, `ΔS` is negative, and thus the term `-TΔS` becomes less negative (or more positive).
- According to the Gibbs free energy equation, `ΔG = ΔH - TΔS`, if `-TΔS` becomes less negative, then `ΔH` must become less negative to maintain the relationship.
- Therefore, this statement is **correct**.
### Step 2: Analyze Statement (b)
**Statement (b):** With the progress of the reaction, the strength of residual forces increases.
- As more gas molecules adsorb onto the surface, the forces acting on the adsorbed molecules do not necessarily increase in strength. Instead, the forces may become balanced.
- The statement implies that the residual forces acting on the adsorbed molecules increase, which is not generally true.
- Therefore, this statement is **incorrect**.
### Step 3: Analyze Statement (c)
**Statement (c):** `NH3` is adsorbed more than `N2`.
- `NH3` is a polar molecule, while `N2` is a non-polar molecule.
- Polar molecules tend to have stronger intermolecular forces and thus are adsorbed more readily on surfaces compared to non-polar molecules.
- Therefore, this statement is **correct**.
### Step 4: Analyze Statement (d)
**Statement (d):** Equilibrium concentration of adsorbate increases with an increase in temperature.
- Adsorption is generally exothermic, meaning that as temperature increases, the equilibrium concentration of adsorbate typically decreases.
- This is because higher temperatures provide more kinetic energy to the molecules, making it harder for them to adhere to the surface.
- Therefore, this statement is **incorrect**.
### Conclusion
The correct statements are (a) and (c).
### Final Answer
The correct statements when adsorption of gas takes place on a metal surface are:
- (a) `ΔH` becomes less negative with the progress of the reaction.
- (c) `NH3` is adsorbed more than `N2`.